If you align the two marks again then you should be set. After aligning them, turn the motor over by hand once to take up any slack in the belt and re-check the alignment. If you want to double check yourself, look in the service manual and it will tell you which marks on the motor to align. If you don't have the manual, look on manualslib.com or similar web site will probably have it.
It's hard to tell from the picture, is that a gouge in the head between the cylinders, or just something white on there? Check both the head and block with a strait edge to be sure they are both flat. If either is not flat then now is the time to fix it. Also if you didn't already, give the cylinders and any moving parts you come across (cams, rockers, etc..) a good liberal smearing with oil. Looks good, let us know how it goes!